文章摘要
王学谦,程晨,马懿星,宁平,徐可,王郎郎,张英杰.直流电晕放电净化羰基硫以及其产物分析[J].材料导报,2017,31(1):149-154
直流电晕放电净化羰基硫以及其产物分析
Removal of Carbonyl Sulfide by DC Corona Discharge and Analysis of the Product
  
DOI：10.11896/j.issn.1005-023X.2017.01.021
中文关键词: 直流电晕等离子体 羰基硫 自由基 尾气
英文关键词: direct current corona plasma, carbonyl sulfide, radical, off-gas
基金项目:国家自然科学基金(51268021;51368026；51568027)；云南省高新技术产业发展项目；西部典型行业环境污染控制协同创新中心开放基金(XTCX2014-05)
作者单位E-mail
王学谦 昆明理工大学环境科学与工程学院,昆明 650093 wxqian3000@aliyun.com 
程晨 昆明理工大学环境科学与工程学院,昆明 650093  
马懿星 昆明理工大学环境科学与工程学院,昆明 650093  
宁平 昆明理工大学环境科学与工程学院,昆明 650093  
徐可 昆明理工大学环境科学与工程学院,昆明 650093  
王郎郎 昆明理工大学环境科学与工程学院,昆明 650093  
张英杰 昆明理工大学环境科学与工程学院,昆明 650093  
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全文下载次数: 2025
中文摘要:
      使用直流电晕放电净化羰基硫(COS),研究不同O2浓度、不同相对湿度以及粉尘存在与否对COS处理效果和被处理后主要产物含量的影响。实验结果表明,随着O2浓度增加,COS去除效率降低,出口气中SO2、总硫(The totals except SO2,记为TS′)生成率均减小,COS转化量与CO、CO2总量保持平衡,CO、CO2浓度降低,CO生成率降低,CO2生成率增加。相对湿度对COS处理效果影响较小,但影响电源击穿电压,相对湿度增加,出口气中总硫生成率增加,SO2生成率减小,出口气中CO生成率降低,而CO2生成率增加,CO浓度降低,CO2浓度增加。在实验过程中加入粉尘后,COS处理效果有一定提高,出口气中SO2生成率显著减少,总硫生成率增加,出口气中CO浓度降低,生成率降低,CO2浓度增加,生成率增加。低氧气浓度、低湿度以及粉尘存在的情况下,COS处理效果最好。
英文摘要:
      The effects of different concentration of O2, different relative humidity and whether if the existence of dust on the concentration of the main product and removal efficiency of carbonyl sulfide (COS) were investigated through direct current corona discharge. The experiment results show that the removal efficiency of carbonyl sulfide (COS) and the production date of sulfur dio-xide (SO2),TS′ were lower with the increase of oxygen(O2); COS inversion quantity was equal to the gross which CO and CO2. The concentration of CO and CO2 were decreased, the production rate of CO was decreased and CO2 was increased. Relative humidity has affected the removal efficiency of COS less,but it has impact on breakdown voltage. With the increase of relative humidity, SO2 formation rate was decreased and TS′ formation rate was increased. The concentration of CO let up and CO2 was increased. The production rate of CO was decreased and CO2 was increased. After add dust in the experiment process, the removal efficiency of COS was increased in some extent, the production rate of SO2 significantly was decreased and TS′ formation rate was in addition. The concentration of CO was decreased and CO2 was increased. The production rate of CO was decreased and CO2 was increased. The remaval efficiency of COS was the best in the condition of low oxygen, low humidity and the exist of dust.
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